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Journal Articles

Operando Br K-edge dispersive X-ray absorption fine structure analysis for Br$$^{-}$$/Br$$_{3}$$$$^{-}$$ redox mediator for Li-Air batteries

Ito, Kimihiko*; Matsumura, Daiju; Song, C.*; Kubo, Yoshimi*

ACS Energy Letters (Internet), 7(6), p.2024 - 2028, 2022/06

 Times Cited Count:2 Percentile:29.01(Chemistry, Physical)

Journal Articles

Development of emergency monitoring system for alpha-particle-emitting radionuclides in the air

Hokama, Tomonori; Fujita, Hiroki; Nakano, Masanao; Iimoto, Takeshi*

Radiation Protection Dosimetry, 196(3-4), p.136 - 140, 2021/11

 Times Cited Count:0 Percentile:0.01(Environmental Sciences)

During the early phase of a nuclear accident, major radioactive materials are released into the environment, necessitating the prompt deployment of various protective actions to avoid or reduce radiation exposure. To implement these actions, the levels of radioactivity in the environment should be determined. However, the radioactivity concentrations of artificial alpha-particle-emitting radionuclides such as plutonium are difficult to measure in airborne samples, because they are interfered with natural radionuclides such as uranium decay products. Therefore, chemical separation is required to measure the concentrations. This study presents a new emergency monitoring system for airborne samples, which performs multiple-pulse time-interval analysis (MTA) without chemical separation. The system is used in conjunction with an alpha/beta-particle survey meter and adopted an analysis method focusing on the detected time interval of each particle. Its features are that a short time to output measurement result, easy handling and nondestructive. The estimated detection limit of the system was 9.5$$times$$10$$^{-2}$$ Bq m$$^{-3}$$. The MTA-based monitoring system could be useful in situations requiring prompt measurement and screening of samples.

Journal Articles

Proposal of evaluation method of graphite incombustibility

Hamamoto, Shimpei; Ohashi, Hirofumi; Iigaki, Kazuhiko; Shimazaki, Yosuke; Ono, Masato; Shimizu, Atsushi; Ishitsuka, Etsuo

Proceedings of 2021 International Congress on Advances in Nuclear Power Plants (ICAPP 2021) (USB Flash Drive), 6 Pages, 2021/10

Since the HTGR has a large amount of graphite material in the core, it is necessary to assume an accident in which the reactor pressure boundary is damaged and air flows into the core. It is important to state that at the time of this accident, graphite does not burn and the accident does not develop due to the heat of oxidation reaction. Therefore, in this study, in order to evaluate the combustibility of graphite materials, we propose a method to compare the calorific value and heat removal amount of the material. When calculating the calorific value, the structural material of HTTR, a high-temperature gas reactor in Japan, was used as a reference. The amount of air in contact with the structural material is a value determined from the chimney effect. The amount of heat release is the sum of convection and radiation. As a result of comparing the heat generation amount with the heat removal amount, it was shown that the heat release amount was always larger than the heat generation amount. This result shows that the graphite material does not depend on the state at the time of the air inflow accident, the temperature decreases and does not burn. It is important to clearly explain the non-flammability of graphite materials when deciding how to deal with severe accidents in HTGRs. This quantitative evaluation method based on a simple theory is considered useful.

Journal Articles

A Portable radioactive plume monitor using a silicon photodiode

Tamakuma, Yuki*; Yamada, Ryohei; Iwaoka, Kazuki*; Hosoda, Masahiro*; Kuroki, Tomohiro*; Mizuno, Hiroyuki*; Yamada, Koji*; Furukawa, Masahide*; Tokonami, Shinji*

Perspectives in Science (Internet), 12, p.100414_1 - 100414_4, 2019/09

In this study, a portable radioactive plume monitor using a silicon photodiode was developed for the detection of a radioactive plume (e.g. $$^{131}$$I, $$^{134}$$Cs and $$^{137}$$Cs) in an emergency situation. It was found that the background count rate was proportional to ambient dose equivalent rate and the detection limit for the monitor at 20 $$mu$$Sv h$$^{-1}$$ as an ambient dose equivalent rate was evaluated to be 187 Bq m$$^{-3}$$ using the ISO11929 method. These results suggest that the detection limit for the system can be decreased effectively by lead shielding with optimized thickness.

Journal Articles

Design approach for mitigation of air ingress in high temperature gas-cooled reactor

Sato, Hiroyuki; Ohashi, Hirofumi; Nakagawa, Shigeaki

Mechanical Engineering Journal (Internet), 4(3), p.16-00495_1 - 16-00495_11, 2017/06

This paper intends to propose a practical solution to protect the HTR from severe oxidation against air ingress accidents without reliance on subsystems. Firstly, a change is made to the center reflector structure to minimize temperature difference during the accident condition in order to reduce buoyancy-driven natural circulation in the reactor. Secondly, a modified structure of the upper reflector is suggested to prevent massive air ingress against a rupture in standpipes. As a preliminary study, a numerical analysis is performed for a typical prismatic-type HTGR. The results showed that amount of air ingress into the reactor can be significantly reduced with practical changes to local structure in the reactor.

Journal Articles

Oxidation behavior of fuel cladding tube in spent fuel pool accident condition

Nemoto, Yoshiyuki; Kaji, Yoshiyuki; Ogawa, Chihiro; Nakashima, Kazuo*; Tojo, Masayuki*

Zairyo To Kankyo, 66(5), p.180 - 187, 2017/05

In spent fuel pool (SFP) under loss-of-cooling or loss-of-coolant severe accident condition, the spent fuels will be exposed to air and heated by their own residual decay heat. Integrity of fuel cladding is crucial for SFP safety therefore study on cladding oxidation in air at high temperature is important. Zircaloy-2 (Zry2) and zircaloy-4 (Zry4) were applied for thermogravimetric analyses (TGA) in different temperatures and different air flow rates in this work. Oxidation rate increased with temperature. In range of air flow rate predicted in spent fuel lack during SFP accident, influence of flow rate was not clearly observed below 950$$^{circ}$$C for Zry2 and below 1050$$^{circ}$$C for Zry4. Over these temperature, oxidation rates appeared obviously higher in higher air flow rate, and this trend became clearer when temperature increased. Oxide layers were carefully examined after the oxidation tests and compared with the mass gain data in TGA to investigate detail of air oxidation process. The results revealed that mass gain data in the pre breakaway transition stage reflects growth of the dense oxide film on specimen surface, and in the post breakaway transition stage, it reflects growth of porous oxide layer beneath the breakaway cracking of the oxide film.

Journal Articles

Design approach for mitigation of air ingress in high temperature gas-cooled reactor

Sato, Hiroyuki; Ohashi, Hirofumi; Nakagawa, Shigeaki

Proceedings of 24th International Conference on Nuclear Engineering (ICONE-24) (DVD-ROM), 8 Pages, 2016/06

This paper intends to propose a practical solution to protect HTGR from severe oxidation against air ingress accidents without reliance on subsystems. Firstly, a change is made to the center reflector structure to minimize temperature difference during the accident condition in order to reduce buoyancy-driven natural circulation in the reactor. Secondly, a modified structure of the upper reflector is suggested to prevent massive air ingress against a rupture in standpipes. As a preliminary study, a numerical analysis is performed for a typical prismatic-type HTGR to study the effectiveness of the proposed design concept using simplified lumped element models. The results showed that amount of air ingress into the reactor can be significantly reduced with practical changes to local structure in the reactor.

Journal Articles

Study on oxidation behavior of cladding for accident conditions in spent fuel pool

Nemoto, Yoshiyuki; Kaji, Yoshiyuki; Ogawa, Chihiro; Nakashima, Kazuo*; Tojo, Masayuki*; Goto, Daisuke*

Fushoku Boshoku Kyokai Dai-62-Kai Zairyo To Kankyo Toronkai Koenshu (CD-ROM), p.23 - 24, 2015/11

In order to clarify the air oxidation behavior of the cladding at high temperatures for study on improvement of safety for accident conditions in spent fuel pool, the oxidation tests for both small specimens under constant temperature conditions and long specimens under loss of coolant simulated temperature conditions were carried out, and the knowledge for influence of both temperature gradient and preoxide film on oxidation behavior of the cladding were obtained in this study.

JAEA Reports

Evaluation of heat exchange performance for air-cooler in HTTR

Tochio, Daisuke; Nakagawa, Shigeaki

JAERI-Tech 2005-041, 109 Pages, 2005/08

JAERI-Tech-2005-041.pdf:4.48MB

In High Temperature Engineering Test Reactor (HTTR) of 30MW, the generated heat at reactor core is finally dissipated at the air-cooler by way of the heat exchangers of the primary pressurized water cooler and the intermediate heat exchanger. To remove generated heat at reactor core and to hold reactor inlet coolant temperature to specified temperature, heat exchangers in main cooling system of HTTR should have designed heat exchange performance. In this report, heat exchange performance for ACL in main cooling system is evaluated with previous operation data, and evaluated values are compared with designed value. Moreover, heat exchange performance at full power operation is estimated for the air temperature. As the result, ACL has heat exchange performance removing generated heat at reactor core under the designe ACL inlet air temperature of 33$$^{circ}$$C.

Journal Articles

High temperature oxidation behavior of titanium beryllide in air

Sato, Yoshiyuki*; Uchida, Munenori*; Kawamura, Hiroshi

JAERI-Conf 2004-006, p.203 - 209, 2004/03

no abstracts in English

JAEA Reports

Estimation of heat removal characteristics for air-cooler in HTTR

Tochio, Daisuke; Nakagawa, Shigeaki; Takada, Eiji*; Sakaba, Nariaki; Takamatsu, Kuniyoshi

JAERI-Tech 2003-097, 55 Pages, 2004/01

JAERI-Tech-2003-097.pdf:3.34MB

In high temperature engineering test reactor (HTTR) of 30 MW, the generated heat at reactor core is finally dissipated at the air-cooler (ACL) by way of the heat exchangers of the primary pressurized water cooler (PPWC) and the intermediate heat exchanger (IHX). Therefore, air temperature (secondary-side condition at ACL) is important factor for the heat removal capability of the reactor. Coping with the air temperature, stable reactor inlet temperature control is achieved by adjusting of ACL coolant temperature with coolant (pressurized water and air) flow rate. ACL heat removal characteristic was based on the previous operation data in rise-to-power test and in-service operation at HTTR. And evaluate heat removal capability at summertime air temperature as the most severe condition was estimated. As the result, it was confirmed that the rated power of 30 MW can be removed at the condition of summertime air-temperature.

Journal Articles

Charged nanoparticle formation from humidified gases with and without dilute benzene under electron beam irradiation

Hakoda, Teruyuki; Kim, H.*; Okuyama, Kikuo*; Kojima, Takuji

Journal of Aerosol Science, 34(8), p.977 - 991, 2003/08

 Times Cited Count:15 Percentile:54.94(Engineering, Chemical)

no abstracts in English

Journal Articles

Characteristics of a simultaneous sampling system for the speciation of atmospheric T and $$^{14}$$C, and its application to surface and soil air

Amano, Hikaru; Koma, T.*; Atarashi-Andoh, Mariko; Koarashi, Jun; Iida, Takao*

Journal of Radioanalytical and Nuclear Chemistry, 252(2), p.353 - 357, 2002/00

 Times Cited Count:6 Percentile:39.54(Chemistry, Analytical)

no abstracts in English

JAEA Reports

Study of technical issues on proton beam line tunnel in material/life science experimental facility of high intensity proton accelerator project

Sakamoto, Shinichi; Meigo, Shinichiro; Konno, Chikara; Harada, Masahide; Miyake, Yasuhiro*; Kasugai, Yoshimi; Muto, Suguru*; Fujimori, Satoru*; Ono, Takehiro; Ikeda, Yujiro

JAERI-Tech 2001-075, 168 Pages, 2001/12

JAERI-Tech-2001-075.pdf:12.78MB

no abstracts in English

JAEA Reports

Radiation control on wastes recovery work in wastes storage pit

Ito, Yasuhisa; Noda, Kimio; ;

JNC TN8410 2001-018, 67 Pages, 2001/04

JNC-TN8410-2001-018.pdf:2.96MB

There are waste storage pits where non-radioactive wastes generated from plutonium fuel facilities were stored in JNC Tokai Works. But radioactive wastes were found in one of the pit during wastes arrangement works. Therefore we set the pit temporary controlled area and recovered wastes from it. This report describes the radiation control technique of recovery work in detail.

JAEA Reports

Radiation monitoring for the HTTR rise-to-power test (1) and (2)'

Nakazawa, Takashi; Yoshino, Toshiaki; Yasu, Katsuji; Ashikagaya, Yoshinobu; Kikuchi, Hisaki

JAERI-Tech 2001-001, 101 Pages, 2001/02

JAERI-Tech-2001-001.pdf:5.15MB

no abstracts in English

JAEA Reports

Improvement of the technique for stack monitoring based on behavior analysis of natural radio-nuclides; The technique for reducing the value of the exhaust monitor's background

Izaki, Kenji; Noda, Kimio; ; Kashimuta, Yoshio*

JNC TN8410 2001-005, 30 Pages, 2001/01

JNC-TN8410-2001-005.pdf:0.62MB

Stack monitoring is the most important work in radiation control works. Exhaust monitors used for stack monitoring have the background (which is the counts by natural radio-nuclides) on normal condition, and the values of the background vary with the facilities. Therefore, if the value of background is high, it is difficult to estimate rapidly the radioactive concentration in the exhaust. In order to estimate rapidly the radioactive concentration in exhaust, we analyzed the behavior of natural radioactivity in the facilities and examine the technique fo reducing the value of the background. As a result of the examination, we found that it is possible to estimate rapidly if we change over the monitoring point to immediately after the HEPA filters on the exhaust duct. In this reports, the analyzed results of behavior of natural radio-nuclides in the facilities and the technique for reducing the values of the background are described. To reduce the value of the background has a major effect on not only rapidly estimating the radioactive density in the exhaust but also finding the unusual things on stack monitoring.

Journal Articles

Numerical analysis on thermal-hydraulic and dust transport behavior in fusion reactors at loss-of-vacuum events

Takase, Kazuyuki

Fusion Engineering and Design, 51-52(Part.B), p.631 - 639, 2000/11

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Study on the passive safe technology for the prevention of air ingress during the primary-pipe rupture accident of HTGR

Takeda, Tetsuaki; Hishida, Makoto*

Nuclear Engineering and Design, 200(1-2), p.251 - 259, 2000/08

 Times Cited Count:26 Percentile:82.67(Nuclear Science & Technology)

no abstracts in English

135 (Records 1-20 displayed on this page)